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Staggered‐grid finite‐difference (FD) schemes are widely used in numerical simulation of seismic wave propagation. The traditional explicit staggered‐grid scheme adopts the second‐order temporal and explicit high‐order spatial FD, so it easily suffers from significant temporal dispersion and the spatial operator–length saturation effect. The recently developed implicit time–space‐domain high‐order staggered‐grid scheme for 2D acoustic wave simulation overcomes those two weaknesses effectively, yielding high‐order accuracies in both time and space and thus better suppressing the numerical dispersion. However, the involved FD coefficients are generally determined by Taylor‐series expansion (TE) or the least‐squares (LS) method and still cannot effectively control spatial dispersion at the large wavenumber range. Adopting the same FD stencil, we alternatively determine the FD coefficients using a combination of TE and the Remez optimization algorithm. The temporal accuracy–related coefficients are determined by the TE of the time–space‐domain dispersion relation, whereas the implicit spatial FD coefficients are calculated by using the Remez exchange optimization algorithm to effectively extend the effective wavenumber range while achieving a high‐order temporal accuracy and consequently enhance the overall modelling accuracy. The newly optimized scheme is then extended into a 3D case. Dispersion and numerical analyses validate that the proposed new schemes better suppress the spatial dispersion while maintaining the high‐order temporal accuracy and outperform the existing TE‐ and LS‐based FD schemes. To further improve the modelling efficiency, the variable–operator–length strategy is combined. Numerical examples of the 2D and 3D complicated models validate the effectiveness of the combined scheme in reducing the operator length and consequently improving the modelling efficiency.