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The Effect of Preferential Nucleation Sites on the Distribution of Secondary Mineral Precipitates
- Publisher: European Association of Geoscientists & Engineers
- Source: Conference Proceedings, 83rd EAGE Annual Conference & Exhibition, Jun 2022, Volume 2022, p.1 - 5
Abstract
Summary
In the process of mineral nucleation and growth, substrate surface properties and substrate types introduce favorable areas where nucleation events are more likely to occur. The preferential sites for mineral nucleation exist because of the lower interfacial free energy between the precipitating phase and the substrate. In this work, we used a pore-scale Lattice Boltzmann (LB)-based reactive transport model incorporated with the developed probabilistic nucleation model in our previous works to investigate the role of the interfacial free energy between the nucleating phase and the substrate on the nucleation and growth of secondary minerals. We also used Shannon entropy to assess the spatial randomness and the evolution path of the systems as solid phases form. The results showed that the developed model can accurately capture the selective behavior of nucleation processes in the presence of preferential sites. The simulation results demonstrate the importance of using a probabilistic nucleation model to capture the correct physics of this phenomenon. It is also concluded that the probabilistic nucleation models are more relevant in environments with longer induction times.
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