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The salars of the Lithium Triangle in South America contain approximately 55% of the world’s lithium resources ( Cabello, 2021 ; Schulz et al., 2017 ). The source, transportation and concentration of the lithium-brines involves a complex mineral system that is dependent upon climate, weathering, basin closure, surface drainage, hydrothermal and groundwater systems, lithium-bearing rock distribution and geological structural control. A suite of satellite platforms, geological datasets, advanced data analytics and automated workflows has enabled the delineation and targeting of potential lithium-rich salars and paleosalars buried beneath recent sediments and volcanics.