1887

Abstract

Summary

Underground hydrogen storage is a highly promising solution for effective utilization of renewable energy resources. By providing the capacity to store surplus energy and balance seasonal supply-demand fluctuations, hydrogen storage is one of the key technologies in achieving a low-carbon energy society. However, the loss of hydrogen from a geologic storage reservoir poses a potential challenge, whether through the caprock, discrete faults or fractures, or through leaky wells.

Faults can act as major structural traps or connect pathways to shallower geological layers, and it is important to understand how hydrogen can migrate through these. Faults are complex geological structures with heterogeneous properties that are challenging to characterize using data acquisition. Petrophysical properties are often derived indirectly, relying on estimations based on other properties. To accurately model and simulate flow through a fault can be both challenging and computationally costly.

We study hydrogen injection into a part of the openly available dataset (co2datashare.org) representing the Smeaheia formation in the North Sea, connected to an overlying aquifer through flow in the Vette fault zone. Efficient computational approaches are used to quantify hydrogen leakage through faults in underground hydrogen storage. A dedicated hydrogen-brine module is implemented in the OPM flow reservoir simulator. Through this module, we perform a comprehensive numerical analysis that examines three crucial aspects: evaluating the influence of upscaled flow functions within a fault, examining the applicability of simplified grid models for a fault located between aquifers, and quantifying leakage of hydrogen through a fault under cyclic injection/production schedule.

This aims to show variation in fault flow, depending on modeling choices such as resolution and flow functions. Additionally, it is evident that utilizing simplified grid models for faults situated between aquifers provides valuable information and highlights that modeling choices are crucial to capture the complete behavior of two-phase flow through faults.

Loading

Article metrics loading...

/content/papers/10.3997/2214-4609.202437059
2024-09-02
2026-03-12
Loading full text...

Full text loading...

References

  1. Batzle, M. and Wang, Z. [1992] Seismic properties of pore fluids.GEOPHYSICS, 57(11), 1396–1408.
    [Google Scholar]
  2. Brooks, R.H. and Corey, A. [1964] Hydraulic properties of porous media.Hydrology Paper, 3.
    [Google Scholar]
  3. Chabab, S., Théveneau, P., Coquelet, C., Corvisier, J. and Paricaud, P. [2020] Measurements and predictive models of high-pressure H2 solubility in brine (H2O+NaCl) for underground hydrogen storage application.International Journal of Hydrogen Energy, 45(56), 32206–32220.
    [Google Scholar]
  4. Daubert, T.E. and Danner, R.P. [1989] Physical and thermodynamic properties of pure chemicals: data compilation. Taylor Francis.
    [Google Scholar]
  5. Dullien, F. [1992] Porous media: fluid transport and pore structure.
    [Google Scholar]
  6. Ferrell, R.T. and Himmelblau, D.M. [1967] Diffusion coefficients of hydrogen and helium in water.AIChE Journal, 13(4), 702–708.
    [Google Scholar]
  7. Flemisch, B., Darcis, M., Erbertseder, K., Faigle, B., Lauser, A., Mosthaf, K., Müthing, S., Nuske, P., Tatomir, A., Wolff, M. and Helmig, R. [2011] DuMux: DUNE for multi-phase, component,scale,physics,... flow and transport in porous media.Advances in Water Resources, 34(9), 1102–1112.
    [Google Scholar]
  8. Garcia, J.E. [2001] Density of aqueous solutions of CO2.No. LBNL-49023, Lawrence Berkeley National Lab. (LBNL), Berkeley, CA.
    [Google Scholar]
  9. Gassnova [2021] Smeaheia CO2 Storage Prospect Reference Dataset.
    [Google Scholar]
  10. Heinemann, N., Alcalde, J., Miocic, J.M., Hangx, S.J.T., Kallmeyer, J., Ostertag-Henning, C., Hassanpouryouzband, A., Thaysen, E.M., Strobel, G.J., Schmidt-Hattenberger, C., Edlmann, K., Wilkinson, M., Bentham, M., Stuart Haszeldine, R., Carbonell, R. and Rudloff, A. [2021] Enabling large-scale hydrogen storage in porous media – the scientific challenges.Energy amp; Environmental Science, 14(2), 853–864.
    [Google Scholar]
  11. Hu, J., Duan, Z., Zhu, C. and Chou, I.M. [2007] PVTx properties of the CO2–H2O and CO2–H2O–NaCl systems below 647 K: Assessment of experimental data and thermodynamic models.Chemical Geology, 238(3), 249–267.
    [Google Scholar]
  12. International Energy Agency [2022] Global Hydrogen Review 2022 – Analysis. Tech. rep., IEA.
    [Google Scholar]
  13. Jafari Raad, S.M., Leonenko, Y. and Hassanzadeh, H. [2022] Hydrogen storage in saline aquifers: Opportunities and challenges.Renewable and Sustainable Energy Reviews, 168, 112846.
    [Google Scholar]
  14. Krevor, S., de Coninck, H., Gasda, S.E., Ghaleigh, N.S., de Gooyert, V., Hajibeygi, H., Juanes, R., Neufeld, J., Roberts, J.J. and Swennenhuis, F. [2023] Subsurface carbon dioxide and hydrogen storage for a sustainable energy future.Nature Reviews Earth amp; Environment, 4(2), 102–118.
    [Google Scholar]
  15. Leachman, J.W., Jacobsen, R.T., Penoncello, S.G. and Lemmon, E.W. [2009] Fundamental Equations of State for Parahydrogen, Normal Hydrogen, and Orthohydrogen.Journal of Physical and Chemical Reference Data, 38(3), 721–748.
    [Google Scholar]
  16. Li, D., Beyer, C. and Bauer, S. [2018] A unified phase equilibrium model for hydrogen solubility and solution density.International Journal of Hydrogen Energy, 43(1), 512–529.
    [Google Scholar]
  17. Lie, K.A. [2019] An Introduction to Reservoir Simulation Using MATLAB/GNU Octave: User Guide for the MATLAB Reservoir Simulation Toolbox (MRST). Cambridge University Press.
    [Google Scholar]
  18. Michaelides, E. [1981] Thermodynamic properties of geothermal fluids.Trans.-Geotherm. Resour. Counc.;(United States), 5(CONF-811015-).
    [Google Scholar]
  19. Miocic, J., Heinemann, N., Edlmann, K., Scafidi, J., Molaei, F. and Alcalde, J. [2023] Enabling Secure Subsurface Storage in Future Energy Systems, chap. Underground hydrogen storage: a review. The Geological Society of London.
    [Google Scholar]
  20. Mouli-Castillo, J., Heinemann, N. and Edlmann, K. [2021] Mapping geological hydrogen storage capacity and regional heating demands: An applied UK case study.Applied Energy, 283, 116348.
    [Google Scholar]
  21. Muzny, C.D., Huber, M.L. and Kazakov, A.F. [2013] Correlation for the Viscosity of Normal Hydrogen Obtained from Symbolic Regression.Journal of Chemical amp; Engineering Data, 58(4), 969–979.
    [Google Scholar]
  22. OPM [2023] OPM Flow Refrence Manual 2023.10.
    [Google Scholar]
  23. Pettersson, P., Keilegavlen, E., Sandve, T.H., Gasda, S. and Krumscheid, S. [2023] Copula modeling and uncertainty propagation in field-scale simulation of CO2 fault leakage.
    [Google Scholar]
  24. Rasmussen, A.F., Sandve, T.H., Bao, K., Lauser, A., Hove, J., Skaflestad, B., Klöfkorn, R., Blatt, M., Rustad, A.B., Sævareid, O., Lie, K.A. and Thune, A. [2021] The Open Porous Media Flow reservoir simulator.Computers & Mathematics with Applications, 81, 159–185.
    [Google Scholar]
  25. Ratcliff, G. and Holdcroft, J. [1963] Diffusivities of gases in aqueous electrolyte solutions.Trans. Inst. Chem. Eng, 41(10), 315–319.
    [Google Scholar]
  26. Ren, B., Jensen, J., Duncan, I. and Lake, L. [2023] Buoyant Flow of H2 Vs. CO2 in Storage Aquifers: Implications to Geological Screening.SPE Reservoir Evaluation amp; Engineering, 26(03), 1048–1058.
    [Google Scholar]
  27. Saeed, M. and Jadhawar, P. [2024] Modelling underground hydrogen storage: A state-of-the-art review of fundamental approaches and findings.Gas Science and Engineering, 121, 205196.
    [Google Scholar]
  28. Sandve, T.H., Gasda, S.E., Rasmussen, A. and Rustad, A.B. [2021] Convective Dissolution in Field Scale Co2 Storage Simulations Using the OPM Flow Simulator. In: TCCS–11. CO2 Capture, Transport and Storage. Trondheim 22nd–23rd June 2021 Short Papers from the 11th International Trondheim CCS Conference.
    [Google Scholar]
  29. Schlumberger [2020] Eclipse Refrence Manual 2020.4.
    [Google Scholar]
  30. Span, R. and Wagner, W. [1996] A New Equation of State for Carbon Dioxide Covering the Fluid Region from the Triple-Point Temperature to 1100 K at Pressures up to 800 MPa.Journal of Physical and Chemical Reference Data, 25(6), 1509–1596.
    [Google Scholar]
  31. Trangenstein, J.A. and Bell, J.B. [1989] Mathematical Structure of the Black-Oil Model for Petroleum Reservoir Simulation.SIAM Journal on Applied Mathematics, 49(3), 749–783.
    [Google Scholar]
/content/papers/10.3997/2214-4609.202437059
Loading
/content/papers/10.3997/2214-4609.202437059
Loading

Data & Media loading...

This is a required field
Please enter a valid email address
Approval was a Success
Invalid data
An Error Occurred
Approval was partially successful, following selected items could not be processed due to error