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The historic Løkken Cu-Zn pyrite mine in Central Norway, active from 1654 to 1987, left behind substantial tailings now being reassessed for their secondary resource potential. As part of a national initiative aligned with EU Critical Raw Materials strategies, the Geological Survey of Norway conducted geophysical surveys in 2023–2024 at the main landfill site using Electrical Resistivity Tomography (ERT) and Ground Penetrating Radar (GPR). ERT, a well-established method for characterizing conductive tailings, proved highly effective in delineating tailings distribution and estimating volume, particularly in the southern portion of the landfill where newer deposits showed low resistivities (<10 Ωm). High-resolution profiling and 2.5D inversion modeling indicated tailings thicknesses of up to 8 meters and an estimated volume of ∼3,160 m3 of conductive material. Although borehole data provided valuable ground truth, no consistent correlation was observed between resistivity and Cu/Zn concentrations. GPR added limited structural detail due to conductive surface layers but aided lateral interpretation through depth slicing. While the methods used are established, the study underscores the importance of optimized, denser ERT profiling to improve spatial coverage and enable the construction of full 3D resistivity models - critical for accurate volume estimation and improved characterization in legacy mine waste assessments.