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Abstract

Summary

In a pilot project in Helguvik, Iceland, in-situ CO mineral storage is tested for the first time using saline water instead of fresh water for injection in the field scale. We present three geophysical and geochemical techniques that are novel to in-situ CO mineral storage site characterization and monitoring. The baseline characterization, employing single-hole electrical resistivity tomography (ERT) and crosshole seismic measurements, revealed decameter-thick basaltic layers and allowed us to interfer the subsurface porosity and permeability distributions. Rock physics modelling predicts significant seismic velocity increases associated with secondary mineral precipitation, suggesting crosshole seismic time-lapse surveys as a valuable monitoring tool. Results of the ERT timelapse measurements show distinct variations between the baseline and the timelapse measurements, indicating potential resistivity changes due to secondary mineral precipitation and fluid substitution. Geochemical monitoring of a Helium tracer confirms that injected water has reached the monitoring well at 100 m distance, whereas the CO concentration in the same well shows no significant increase relative to the pre-injection state. This work demonstrates the potential of combined geophysical and geochemical methods for characterizing and monitoring in-situ CO mineral storage, highlighting ERT and crosshole seismics as valuable tools.

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2025-09-01
2026-02-14
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References

  1. Aradóttir, E. S. P., Sonnenthal, E. L., Björnsson, G., and Jónsson, H. [2012]. Multidimensional reactive transport modeling of CO2 mineral sequestration in basalts at the Hellisheidi geothermal field, Iceland. International Journal of Greenhouse Gas Control, 9, 24–40. https://doi.org/10.1016/j.ijggc.2012.02.006
    [Google Scholar]
  2. Archie, G. E. [1942]. The Electrical Resistivity Log as an Aid in Determining Some Reservoir Characteristics. Transactions of the AIME, 146(01), 54–62. https://doi.org/10.2118/942054-G.
    [Google Scholar]
  3. Bachmann, F., Hielscher, R., and Schaeben, H. [2010]. Texture Analysis with MTEX – Free and Open Source Software Toolbox. Solid State Phenom., 160, 63–68. https://doi.org/10.4028/www.scientific.net/SSP.160.63
    [Google Scholar]
  4. Bellezza, C., Barison, E., Farina, B., Poletto, F., Meneghini, F., Böhm, G., Dragonov, D., Janssen, M.T., van Otten, G., Stork, A.L., Chalari, A., Schleifer, A., Durucan, S. [2024]. Multi-sensor seismic processing approach using geophones and HWC DAS in the monitoring of CO2 storage at the Hellisheiði geothermal field in Iceland. Sustainability: Science Practice and Policy, 16(2), 877. https://doi.org/10.3390/su16020877
    [Google Scholar]
  5. Brennwald, M. S., Schmidt, M., Oser, J., and Kipfer, R. [2016]. A portable and autonomous mass spectrometric system for on-site environmental gas analysis. Environmental Science & Technology, 50(24), 13455–13463. https://doi.org/10.1021/acs.est.6b03669
    [Google Scholar]
  6. Gassmann, F. [1951]. Ueber die Elastizität poröser Medien [Book]. Zürich: Institut für Geophysik.
    [Google Scholar]
  7. Hassing, S. H. W., Draganov, D., Janssen, M., Barnhoorn, A., Wolf, K. -H A. A., van den Berg, J., Friebel, M., van Otten, G., Poletto, F., Bellezza, C., Barison, E., Brynjarsson, B., Hjörleifsdóttir, V., Obermann, A., Sánchez-Pastor, P., Durucan, S. [2024]. Imaging CO 2 reinjection into basalts at the CarbFix2 reinjection reservoir (Hellisheiði, Iceland) with body‐wave seismic interferometry. Geophysical Prospecting, 1–5. https://doi.org/10.1111/1365-2478.13472
    [Google Scholar]
  8. Junker, J. S., Obermann, A., Voigt, M., Maurer, H., Eruteya, O. E., Moscariello, A., Wiemer, S., and Zappone, A. [2025]. Geophysical characterization of the in-situ CO2 mineral storage pilot site in Helguvik, Iceland. International Journal of Greenhouse Gas Control, 141(104320), 104320. https://doi.org/10.1016/j.ijggc.2025.104320
    [Google Scholar]
  9. Lévy, L., Maurya, P. K., Byrdina, S., Vandemeulebrouck, J., Sigmundsson, F., Árnason, K., Ricci, T., Deldicque, D., Roger, M., Gibert, B., Labazuy, P. [2019]. Electrical resistivity tomography and time-domain induced polarization field investigations of geothermal areas at Krafla, Iceland:comparison to borehole and laboratory frequency-domain electrical observations. Geophysical Journal International, 218(3), 1469–1489. https://doi.org/10.1093/gji/ggz240
    [Google Scholar]
  10. Marieni, C., Voigt, M., Clark, D. E., Gíslason, S. R., and Oelkers, E. H. [2021]. Mineralization potential of water-dissolved CO2 and H2S injected into basalts as function of temperature: Freshwater versus Seawater. International Journal of Greenhouse Gas Control, 109, 103357. https://doi.org/10.1016/J.IJGGC.2021.103357
    [Google Scholar]
  11. Matter, J. M., Stute, M., Snæbjörnsdóttir, S. Ó., Oelkers, E. H., Gislason, S. R., Aradóttir, E. S. P., Sigfússon, B., Gunnarsson, I., Sigurdardottir, H., Gunnlaugsson, E., Axelsson, G., Alfredsson, H. A., Wolff-Boenisch, D., Mesfin, K., Taya, D. F., Hall, J., Dideriksen, K, Broecker, W. S. [2016]. Rapid carbon mineralization for permanent disposal of anthropogenic carbon dioxide emissions. Science, 352(6291), 1312–1314. https://doi.org/10.1126/science.aad8132
    [Google Scholar]
  12. Snæbjörnsdóttir, S. Ó., Gislason, S. R., Galeczka, I. M., and Oelkers, E. H. [2018]. Reaction path modelling of in-situ mineralisation of CO2 at the CarbFix site at Hellisheidi, SW-Iceland. Geochimica et Cosmochimica Acta, 220, 348–366. https://doi.org/10.1016/j.gca.2017.09.053
    [Google Scholar]
  13. Snæbjörnsdóttir, S. Ó., Sigfússon, B., Marieni, C., Goldberg, D. S., Gislason, S. R., and Oelkers, E. H. [2020]. Carbon dioxide storage through mineral carbonation. Nature Reviews Earth & Environment, 1(2), 90–102. https://doi.org/10.1038/s43017-019-0011-8
    [Google Scholar]
  14. Stavropoulou, E. [2024]. Impact of CO2-rich seawater injection on the flow properties of basalts [Data set]. https://doi.org/10.5281/ZENODO.10910996
    [Google Scholar]
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